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Space is the Place is awesome. Both of them. (the album and the soundtrack to the film)
I think I have heard Atlantis but don't remember loving it all that much. Some good Sun Ra ones are, in my opinion:
Outerspaceways Incorporated (a live set from 68, I think, which mixes the swinging stuff with the more out there stuff)
Cosmic Tones for Mental Therapy
Art Forms of Dimension Tomorrow
Heliocentric Worlds vol1 and 2
The Solar Myth Approach vol 1 and 2 (these are pretty out there)
Nuclear War
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